TY - JOUR
T1 - Portable point-of-use photoelectrocatalytic device provides rapid water disinfection
AU - Montenegro-Ayo, Renato
AU - Barrios, Ana C.
AU - Mondal, Indrayudh
AU - Bhagat, Kartik
AU - Morales-Gomero, Juan Carlos
AU - Abbaszadegan, Morteza
AU - Westerhoff, Paul
AU - Perreault, François
AU - Garcia-Segura, Sergi
N1 - Publisher Copyright:
© 2020 Elsevier B.V.
PY - 2020/10/1
Y1 - 2020/10/1
N2 - Portable water purification devices are needed to provide safe drinking water in rural communities, developing communities with low quality centralized water distribution, and military or recreational applications. Filtration, ultraviolet light, or chemical additives provide a spectrum of alternatives to remove pathogens from water. For the first time, we design, fabricate and demonstrate the performance of a small portable photoelectric point-of-use device, and document its performance on pathogen inactivation. The device utilizes a commercial teacup from which TiO2 nanotube photoanodes were produced in-situ and, with a small rechargeable battery powered 365 nm light emitting diode, was able to achieve 5-log inactivation of Escherichia coli in 10 s and 2.6-log of Legionella in 60 s of treatment in model water samples. Treatment of natural water achieved a 1-log bacteria inactivation after 30 s due to matrix effects. The electro-photocatalytic disinfection reactor in a kup (e-DRINK) can provide a feasible and affordable solution to ensure access to clean water. More broadly, this work demonstrates the potential for illumination to improve the efficiency of electrocatalytic surfaces.
AB - Portable water purification devices are needed to provide safe drinking water in rural communities, developing communities with low quality centralized water distribution, and military or recreational applications. Filtration, ultraviolet light, or chemical additives provide a spectrum of alternatives to remove pathogens from water. For the first time, we design, fabricate and demonstrate the performance of a small portable photoelectric point-of-use device, and document its performance on pathogen inactivation. The device utilizes a commercial teacup from which TiO2 nanotube photoanodes were produced in-situ and, with a small rechargeable battery powered 365 nm light emitting diode, was able to achieve 5-log inactivation of Escherichia coli in 10 s and 2.6-log of Legionella in 60 s of treatment in model water samples. Treatment of natural water achieved a 1-log bacteria inactivation after 30 s due to matrix effects. The electro-photocatalytic disinfection reactor in a kup (e-DRINK) can provide a feasible and affordable solution to ensure access to clean water. More broadly, this work demonstrates the potential for illumination to improve the efficiency of electrocatalytic surfaces.
KW - Electrochemical advanced oxidation processes
KW - Escherichia coli
KW - Legionella
KW - TiO nanotubes photo-anodes
KW - Translational technology
KW - Water treatment
UR - https://hdl.handle.net/20.500.12724/11107
UR - http://www.scopus.com/inward/record.url?scp=85087389268&partnerID=8YFLogxK
U2 - 10.1016/j.scitotenv.2020.140044
DO - 10.1016/j.scitotenv.2020.140044
M3 - Artículo (Contribución a Revista)
AN - SCOPUS:85087389268
SN - 0048-9697
VL - 737
JO - Science of the Total Environment
JF - Science of the Total Environment
M1 - 140044
ER -